Li, Hui; Schubert, C.; Dral, P. O.; Costa, R. D.; La Rosa, A.; Thüring, Jürg; Liu, Shi-Xia; Yi, Chenyi; Filippone, S.; Martin, N.; Decurtins, Silvio; Clark, T.; Guldi, D. M. (2013). Probing Charge Transfer in Benzodifuran-C-60 Dumbbell-Type Electron Donor-Acceptor Conjugates: Ground- and Excited-State Assays. ChemPhysChem, 14(13), pp. 2910-2919. Wiley-VCH 10.1002/cphc.201300378
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Rigid electron donor-acceptor conjugates (1-3) that combine -extended benzodifurans as electron donors and C-60 molecules as electron acceptors with different linkers have been synthesized and investigated with respect to intramolecular charge-transfer events. Electrochemistry, fluorescence, and transient absorption measurements revealed tunable and structure-dependent charge-transfer processes in the ground and excited states. Our experimental findings are underpinned by density-functional theory calculations.
Item Type: |
Journal Article (Original Article) |
|---|---|
Division/Institute: |
08 Faculty of Science > Department of Chemistry, Biochemistry and Pharmaceutical Sciences (DCBP) |
UniBE Contributor: |
Li, Hui, Liu, Shi-Xia, Yi, Chenyi, Decurtins, Silvio |
Subjects: |
500 Science > 570 Life sciences; biology 500 Science > 540 Chemistry |
ISSN: |
1439-4235 |
Publisher: |
Wiley-VCH |
Language: |
English |
Submitter: |
Gabriela Claudia Frei |
Date Deposited: |
29 Jul 2014 08:41 |
Last Modified: |
05 Dec 2022 14:31 |
Publisher DOI: |
10.1002/cphc.201300378 |
PubMed ID: |
23918655 |
Uncontrolled Keywords: |
benzodifuran, cyclovoltammetry, donor–acceptor systems, fullerenes, photophysics |
BORIS DOI: |
10.7892/boris.46367 |
URI: |
https://boris.unibe.ch/id/eprint/46367 |
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